Centuries-Old Smoke Particles Preserved in Ice Reveal a Fiery Past – And the Future of Global Climate Change

Wildfires on the Patagonian Steppe

Smoke from human-caused wildfires on the Patagonian steppe are trapped in Antarctic ice. Credit: Kathy Kasic/Brett Kuxhausen, Montana State University

Ice core samples reveal significant smoke aerosols in the pre-industrial Southern Hemisphere.

Centuries-old smoke particles preserved in the ice reveal a fiery past in the Southern Hemisphere and shed new light on the future impacts of global climate change, according to new research published in Science Advances.

“Up till now, the magnitude of past fire activity, and thus the amount of smoke in the preindustrial atmosphere, has not been well characterized,” said Pengfei Liu, a former graduate student and postdoctoral fellow at the Harvard John A. Paulson School of Engineering and Applied Sciences (SEAS) and first author of the paper. “These results have importance for understanding the evolution of climate change from the 1750s until today, and for predicting future climate.”

One of the biggest uncertainties when it comes to predicting the future impacts of climate change is how fast surface temperatures will rise in response to increases in greenhouse gases. Predicting these temperatures is complicated since it involves the calculation of competing warming and cooling effects in the atmosphere. Greenhouse gases trap heat and warm the planet’s surface while aerosol particles in the atmosphere from volcanoes, fires and other combustion cool the planet by blocking sunlight or seeding cloud cover. Understanding how sensitive surface temperature is to each of these effects and how they interact is critical to predicting the future impact of climate change.

Ice Core Sample

Ancient ice from James Ross Island in the Northern Antarctic Peninsula about to be extracted from the drill barrel. Credit: Robert Mulvaney

Many of today’s climate models rely on past levels of greenhouse gasses and aerosols to validate their predictions for the future. But there’s a problem: While pre-industrial levels of greenhouse gasses are well documented, the amount of smoke aerosols in the preindustrial atmosphere is not.

To model smoke in the pre-industrial Southern Hemisphere, the research team looked to Antarctica, where the ice trapped smoke particles emitted from fires in Australia, Africa, and South America. Ice core scientists and co-authors of the study, Joseph McConnell and Nathan Chellman from the Desert Research Institute in Nevada, measured soot, a key component of smoke, deposited in an array of 14 ice cores from across the continent, many provided by international collaborators.

“Soot deposited in glacier ice directly reflects past atmospheric concentrations so well-dated ice cores provide the most reliable long-term records,” said McConnell.

What they found was unexpected.

“While most studies have assumed less fire took place in the preindustrial era, the ice cores suggested a much fierier past, at least in the Southern Hemisphere,” said Loretta Mickley, Senior Research Fellow in Chemistry-Climate Interactions at SEAS and senior author of the paper.

Pengfei Liu and Nathan Chellman

Pengfei Liu (left) and Nathan Chellman with an ice core sample. Credit: Pengfei Liu

To account for these levels of smoke, the researchers ran computer simulations that account for both wildfires and the burning practices of indigenous people.

“The computer simulations of fire show that the atmosphere of the Southern Hemisphere could have been very smoky in the century before the Industrial Revolution. Soot concentrations in the atmosphere were up to four times greater than previous studies suggested. Most of this was caused by widespread and regular burning practiced by indigenous peoples in the pre-colonial period,” said Jed Kaplan, Associate Professor at the University of Hong Kong and co-author of the study.

This result agrees with the ice core records that also show that soot was abundant before the start of the industrial era and has remained relatively constant through the 20th century. The modeling suggests that as land use changes decreased fire activity, emissions from industry increased.

What does this finding mean for future surface temperatures?

By underestimating the cooling effect of smoke particles in the pre-industrial world, climate models might have over-estimated the warming effect of carbon dioxide and other greenhouse gasses in order to account for the observed increases in surface temperatures.

“Climate scientists have known that the most recent generation of climate models have been over-estimating surface temperature sensitivity to greenhouse gasses, but we haven’t known why or by how much,” said Liu. “This research offers a possible explanation.”

“Clearly the world is warming but the key question is how fast will it warm as greenhouse gas emissions continue to rise. This research allows us to refine our predictions moving forward,” said Mickley.

Reference: “Improved estimates of preindustrial biomass burning reduce the magnitude of aerosol climate forcing in the Southern Hemisphere” by Pengfei Liu, Jed O. Kaplan, Loretta J. Mickley, Yang Li, Nathan J. Chellman, Monica M. Arienzo, John K. Kodros, Jeffrey R. Pierce, Michael Sigl, Johannes Freitag, Robert Mulvaney, Mark A. J. Curran and Joseph R. McConnell, 28 May 2021, Science Advances.
DOI: 10.1126/sciadv.abc1379 

The research was co-authored by Yang Li, Monica Arienzo, John Kodros, Jeffrey Pierce, Michael Sigl, Johannes Freitag, Robert Mulvaney and Mark Curran.

It was funded by the National Science Foundation’s Geosciences Directorate under grants AGS-1702814 and 1702830, with additional support from 0538416, 0538427, and 0839093.

2 Comments on "Centuries-Old Smoke Particles Preserved in Ice Reveal a Fiery Past – And the Future of Global Climate Change"

  1. Clyde Spencer | June 18, 2021 at 12:11 pm | Reply

    “Many of today’s climate models rely on past levels of greenhouse gasses and aerosols to validate their predictions for the future.”

    There is a problem here in that, on a geological time-scale, there is poor correlation between CO2 and temperatures, and the evidence often suggests that warming caused increased CO2, the opposite of what the models assume. Currently, there appears to be strong correlation between CO2 and average temperatures; however, one has to be careful about spurious correlations!

    It is obvious that significant temperature changes took place before industrialization! Antarctic ice cores, such as from Law Dome, strongly suggest that temperatures rose about 800 years before the CO2 levels increased.

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