Ions in the Machine: Performing Complex Calculations Using Simple Liquids Like Water

Researchershave developed a novel reservoir computing system utilizing electrochemical reactions in Faradic current.

This system, tested with different ionic solutions, shows promise for advanced computational tasks by leveraging the unique properties of electrochemical ion reactions for more efficient and cost-effective computing.

After many decades of astonishing developments, advances in semiconductor-based computing are beginning to slow as transistors reach their physical limits in size and speed. However, the requirements for computing continue to grow, especially in artificial intelligence, where neural networks often have several millions of parameters. One solution to this problem is reservoir computing, and a team of researchers led by Osaka University, with colleagues from the University of Tokyo and Hokkaido University, have developed a simple system based on electrochemical reactions in Faradic current that they believe will jump-start developments in this field. 

The Core of Reservoir Computing Systems

Reservoir computing is a relatively recent idea in computing. Instead of traditional binary programs run on semiconductor chips, the reactions of a nonlinear dynamical system—the reservoir—are used to perform much of the calculation. Various nonlinear dynamical systems from quantum processes to optical laser components have been considered as reservoirs. In this study, the researchers looked at the ionic conductance of electrochemical solutions.

“Our simple testing device consists of 90 pairs of planar electrodes with an ionic solution dropped on its surface,” explains Professor Megumi Akai-Kasaya, lead author of the study. “The response voltage to the input voltage is then used as the response of the reservoir.” This voltage response is due to both the ionic currents that pass through the solution and the electrochemical current. This input–output relationship is both nonlinear and reproducible, which makes it suitable for use in reservoir computing. A unique multiway data acquisition system on the device controls the readout nodes, which enables parallel testing.

Evaluating Performance and Potential Applications

The researchers used the device to evaluate two liquids: polyoxometalate molecules in solution and deionized water. The system displayed a “feedforward connection” between nodes, regardless of which sample was used. However, there were differences. “The polyoxometalate solution increased the diversity of the response current, which makes it good at predicting periodic signals,” says Professor Akai-Kasaya. “But it turns out that deionized water is best for solving second-order nonlinear problems.” The good performance of these solutions demonstrates their potential for more complicated tasks, such as handwriting font recognition, isolated word recognition, and other classification tasks.

Potential for Advanced Electrochemical Computing

The researchers believe that proton or ion transfer with minimal electrochemical reactions over short durations has the potential for development as a more computationally powerful computing system that is low in cost and energy efficient. The simplicity of the proposed system opens up exciting new opportunities for developing computing systems based on electrochemical ion reactions.

Reference: “Physical Implementation of Reservoir Computing through Electrochemical Reaction” by Shaohua Kan, Kohei Nakajima, Tetsuya Asai and Megumi Akai-Kasaya, 29 December 2021, Advanced Science.
DOI: 10.1002/advs.202104076

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